Optical Momentum – Lectures

My latest research grant from ANRF is on “Opto-Thermal Binding of Plasmonic Matter”. This is a topic that is at the interface of optical momentum, thermodynamics, statistical physics, and advanced optical microscopy in the real and momentum spaces.

Optical momentum and its measurement have a rich history in understanding electromagnetic waves and their interaction with matter. Over the past century, multiple applications have emerged that harness the transfer of momentum from light to matter. Interestingly, the light that is scattered off this interaction also carries relevant information not only about the interaction but also about certain parameters of light and the participating matter.

These lectures are my attempt to give an overview of the field. My main target audience is my PhD group members and senior undergraduates who are working with me. But these lectures can be followed by anyone who is seriously interested in physics. The discussion involves theoretical optical physics (including elements of statistical and quantum optics), experimental techniques (including advanced microscopy methods) and a few computational techniques connected to the interaction. The goal of the lectures is to reveal the interesting questions in research papers, review articles, monographs and conference papers related to the field and their possible application in industries, including biophotonics and astro and space-photonics. From time to time, I will also discuss our research results from the project.

Light pressure – Lebedev coin

Today, in my optics class, I discussed optical forces due to momentum in electromagnetic waves. Towards the late 1800s, it was realized that light can impart momentum. This manifested as radiation pressure in the electromagnetic theory proposed by James Maxwell.

Pyotr Nikolaevich Lebedev (24 February 1866 – 1 March 1912) was one of the earliest to experimentally measure (~1899) the radiation pressure on a surface (link to his 1900 paper in German). In 1991, the Soviet Union released a 1 ruble coin (pictured above) to commemorate Lebedev’s scientific achievement.

The formula expresses the total momentum transferred per unit time ( radiation pressure, P) by a beam of N photons, each of energy hν, that is incident on a surface with a coefficient of reflectivity ρ. The constant, c, is the speed of light.

The discussion in the class was mainly related to Ashkin’s work. I have written about this in the past.

Shared below is a delightful lecture given by Ashkin at the age of ~96, after he received his Nobel prize.

Art and Chu – in Bell labs

Steven Chu and Arthur Ashkin in 1986, in front of the apparatus shortly after the first optical trapping experiment was completed. Image from Chu’s Nobel lecture.

Steven Chu’s Nobel lecture has some gems. Below, he shares his experience of working with Arthur Ashkin.

“In 1986, the world was excited about atom trapping. During this time, Art Ashkin began to use optical tweezers to trap micron sized particles. While experimenting with colloidal tobacco mosaic viruses, he noticed tiny, translucent objects in his sample. Rushing into my lab, he excitedly proclaimed that he had ‘discovered Life’. I went into his lab, half thinking that the excitement of the last few years had finally gotten the better of him. In his lab was a microscope objective focusing an argon laser beam into a petri dish of water. Off to the side was an old Edmund Scientific microscope. Squinting into the microscope, I saw my eye lashes. Squinting harder, I occasionally saw some translucent objects. Many of these objects were ‘floaters’, debris in my vitreous humor that could be moved by blinking my eyes. Art assured me that there were other objects there that would not move when I blinked my eyes. Sure enough, there were objects in the water that could be trapped and would swim away if the light were turned off. Art had discovered bugs in his apparatus, but these were real bugs, bacteria that had eventually grown in his sample beads and water.”

Chu won the physics Nobel in 1997, and Ashkin won the same in 2018. Ashkin was the pioneer of optical trapping and tweezers, and applied it to a variety of problems, including the manipulation of biological matter. Chu harnessed the momentum of light to trap and cool atoms. Both started their work and collaborated at Bell Labs. Chu moved to Stanford, whereas Ashkin stayed back. Bell Labs was a remarkable place in the 1980s, as Chu describes in his lecture :

“Bell Labs was a researcher’s paradise. Our management supplied us with funding, shielded us from bureaucracy, and urged us to do the best science possible. The cramped labs and office cubicles forced us to rub shoulders with each other. Animated discussions frequently interrupted seminars and casual conversations in the cafeteria would sometimes mark the beginning of a new collaboration.”

Can the world afford to have another Bell Labs in 2025? Can it recreate the magic?

Optothermally induced active & chiral motion – a new paper

We have a new paper in Soft Matter

link to the paper (free to access, thanks to IISER Pune library)

We use optical illumination to generate thermal fields, creating non-reciprocal interactions between passive and active colloids. Active colloids absorb light and produce thermal gradients, driving thermo-osmotic forces that induce propulsion and chiral motion. Our Langevin simulations, backed by experimental observation, reveal how to control colloidal behavior. May have implications in light-driven chiral motion and nonlinear dynamics.

Super effort by Rahul, Ashutosh & Sneha from our group, who combined numerical simulations, analytical theory, with experimental observations.

The 2 anonymous reviewers made us think and work hard, and we thank them!

Also, the paper is part of the journal’s themed collection on “Colloidal interactions, dynamics and rheology”

Gold nanoparticles in sync – preprint

We have a new preprint: https://arxiv.org/abs/2411.15512

The central circle indicates anchored gold nanoparticles stuck to the glass, and the two moving circles are gold colloids that are trapped synchronously due to the optothermal potential.

Optothermal revolution – preprint

We have an Arxiv preprint on how a mixture of colloids (thermally active + passive particles in water) can lead to the emergence of revolution dynamics in an optical ring trap (dotted line). Super effort by our lab members Rahul Chand and Ashutosh Shukla.

Interestingly, the revolution emerges only when an active and a passive colloid are combined (not as individuals) in a ring potential (dotted line)

the direction (clock or anti-clockwise) of the revolution depends on the relative placement of the colloids in the trap

This revolution can be further used to propel a third active colloid

There are many more details in the paper. Check it out: https://arxiv.org/abs/2409.16792